在CW-MFC中的铁基阳极:污染物清除和硫甲醇消除的机制和性能提升
Feng Liu1, Panpan Cui1, Yun Zhang1
1School of Chemistry and Chemical Engineering, Jiangxi Science and Technology Normal University,Nanchang, Jiangxi 330013, PR China.
Bioelectrochemistry (Amsterdam, Netherlands)
|November 29, 2025
概括
建筑湿地微生物燃料电池 (CW-MFCs) 中的铁改性阳极显著提高了抗生素的去除和发电. 这项研究强调以铁为基础的生物炭是有效的废水处理和能量回收的优质阳极材料.
科学领域:
- 环境科学 环境科学
- 环境工程 环境工程
- 微生物学 微生物学
背景情况:
- 建造的湿地微生物燃料电池 (CW-MFCs) 对抗生素去除有希望.
- 阳极材料极大地影响了CW-MFC的性能.
- 硫甲醇 (SMX) 是一种常见的抗生素污染物.
研究的目的:
- 调查活性炭,基于铁的生物炭和酸盐阳极对CW-MFC性能的影响.
- 为了评估污染物去除,发电和微生物社区转移.
- 为了确定CW-MFCs中铁修正的有效性.
主要方法:
- 三种阳极材料的比较:活性炭 (ACCW-MFC),基于铁的生物炭 (FCW-MFC) 和铁矿石 (PCW-MFC).
- 对化学氧气需求 (COD),总 (TP) 和SMX的去除效率的评估.
- 监测发电和分析微生物群落组成.
主要成果:
- FCW-MFC实现了高清除率:96.4%的COD,100%的TP和100%的SMX.
- FCW-MFC表现出对冲击负载的优越弹性.
- PCW-MFC显示高峰电压为402mV (SMX前) 和399mV (SMX后).
- Pseudomonadota 在微生物群落中占主导地位;FCW-MFC 和 PCW-MFC 丰富了无化的 Thauera 属.
结论:
- 在CW-MFC阳极中铁的补充显著增强了电活性微生物群落.
- 基于铁的生物炭和酸盐阳极提高了CW-MFC在污染物清除和能量回收方面的整体性能.
- 带有铁修改阳极的CW-MFC提供了一种有效的策略,可以同时处理废水和发电.
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