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在碳基材料中微调含氧的功能组,用于电催化反应

Xinyu Zheng¹, Guanbin Ding¹, Qiannan Li¹

¹State Key Laboratory of Pollution Control and Resources Reuse, School of Environmental Science and Engineering, Tongji University, Shanghai, 200092, P. R. China.

Chemphyschem : a European journal of chemical physics and physical chemistry

|December 12, 2025

概括

氧功能组 (OFG) 增强碳基电催化剂,以实现可持续能源. 本综述详细介绍了OFG如何改善电催化反应,如减少氧气和减少二氧化碳,为高效的能源解决方案铺平道路.

科学领域:

材料科学材料科学材料科学
电化学电化学电化学
催化剂是一种催化剂.

背景情况:

电催化技术对于满足全球能源需求和实现碳中和至关重要.
碳基材料是有前途的电催化剂,因为它们的有利性质,但它们的惰性结构限制了活性.
将氧功能组 (OFG) 纳入碳材料是提高电催化性能的一个关键策略.

研究的目的:

系统地审查对碳基电催化剂中OFG的最新研究.
探索OFG调节电催化反应的机制,包括氧气减少,二氧化碳减少和氧气演变.
总结结构-功能关系,并讨论OFG改性碳材料的未来机会.

主要方法:

关于电催化剂氧功能组的最新进展的文献综述.
分析受OFG影响的反应动力学和电荷转移过程.
在多反应系统中研究各种OFG类型的结构-属性相关性.

主要成果:

其他催化剂有效调整碳基电催化剂的电子结构,电荷转移和吸附能.
特定的OFG在关键的电催化反应 (氧气减少,二氧化碳减少,氧气演变) 中表现出显著的增强.
精确的对OFG的控制可以提高电催化活性和稳定性.

结论:

在克服电催化用惰性碳结构的局限性方面,OFG是关键的.
了解OFG的精确结构功能关系对于设计高性能电催化剂至关重要.
未来的研究应该集中在可控制的OFG调制策略和用于先进的电催化应用的接口工程.

关键词:

减少二氧化碳的减少碳基材料是基于碳的材料.氧气的进化氧气的进化氧气功能组是指氧气的功能组.减少氧气减少氧气

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