揭示土壤-大米-人类通路上的重金属的命运:源-水槽量化,根球过程和健康影响
Qiumei Wu1, Wenyou Hu2, Shiyi Zhang3
1State Key Laboratory of Soil and Sustainable Agriculture, Institute of Soil Science, Chinese Academy of Sciences, Nanjing 211135, China; Sino-Danish Center for Education and Research (SDC), University of Chinese Academy of Sciences, Beijing 100049, China; Department of Plant and Environmental Sciences, University of Copenhagen, 1871 Frederiksberg C, Denmark.
Journal of hazardous materials
|January 20, 2026
概括
工业和农业的增长增加了农田中的重金属 (HM),对食品安全构成风险. 本研究量化了 (Cd) 暴露和健康风险,确定了影响积累和吸收的关键土壤因素和人类活动.
科学领域:
- 环境科学 环境科学
- 土壤科学 土壤科学
- 毒理学 毒理学 毒理学
背景情况:
- 工业和农业的强化增加了重金属 (HM) 投入到农田,增加了对土壤作物系统和人类健康的风险.
- 在土壤-作物-人类系统中对HM污染的准确评估受到有限的源-下水槽流量数据和暴露估计的阻碍.
研究的目的:
- 研究工业和农业强化对农田HM污染的影响,特别关注 (Cd) 对人类健康的风险.
- 评估饮食中的Cd暴露,并确定影响Cd积累和严重受影响的流域中人类健康风险的关键因素.
主要方法:
- 综合重金属 (HM) 流量监测, (Cd) 生物可访问性分析,社会经济和地理数据以及健康风险建模.
- 利用Cd同位素分析,机器学习 (XGBoost) 和两阶段回归来识别主导的Cd来源,沉积点和调节因素.
- 在人口密,人为影响的流域中评估饮食中的Cd暴露.
主要成果:
- 土壤样本显示Cd污染,15.5%超过了中国的风险值;大气沉积和作物收获是主要的Cd来源和沉积点.
- 机器学习确定了米Cd生物度因子 (CdB),土壤pH,有机物质 (SOM) 和阴离子交换能力 (CEC) 作为人类健康风险的关键预测因素.
- 土壤的pH,CEC和SOM调节了CdB,而根表面的铁斑组成则通过氧化还原敏感通道影响了Cd的吸收.
结论:
- 这项研究通过整合源分配,根球过程和人类暴露,为区域范围的风险评估提供了一种新的方法.
- 这些发现为有针对性的污染控制战略和可持续农业管理提供了关键的见解,以减轻重金属风险.
- 了解土壤特性,植物吸收和人类暴露之间的相互作用对于管理农业系统中的污染至关重要.
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