Principles and performance of an electron spin echo spectrometer using far infrared lasers as excitation sources

We have built an electron spin echo spectrometer operating at 604 GHz, extending the frequency limit of existing spectrometers by more than a factor of 4. In order to handle this high frequency we have used optical techniques, i.e., molecular gas lasers for the excitation pulses and far infrared techniques for the heterodyne detection system. The different components of the spectrometer are described in detail and first experimental results are given.