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Updated: Jul 19, 2026

All-electronic Nanosecond-resolved Scanning Tunneling Microscopy: Facilitating the Investigation of Single Dopant Charge Dynamics
Published on: January 19, 2018
Extreme ultrafast dynamics of quasiparticles excited in surface electronic bands
P Lazić1, V M Silkin, E V Chulkov
1Donostia International Physics Center, E-20018 San Sebastian, Spain.
Abstract:
We develop a many-body description of the nonadiabatic dynamics of quasiparticles in surface bands valid on an extremely ultrashort time scale by combining the formalism for the calculation of quasiparticle survival probabilities with the self-consistent treatment of the electronic response of the system. Applying this approach to the benchmark Cu(111) surface, we assess the behavior and intervals of preasymptotic electron and hole dynamics in surface bands and locate the transition to the asymptotic regime of the exponential quasiparticle decay characterized by the corrected Fermi golden rule-type of transition rate. The general validity of these findings enables distinguishing the various regimes of ultrafast electron dynamics that may be revealed in time resolved experiments.
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