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Updated: Jul 9, 2026

10:52
Direct Imaging of Laser-driven Ultrafast Molecular Rotation
Published on: February 4, 2017
Optical frequency conversion by a rotating molecular wave plate
Optics Letters
|November 28, 2007
Abstract:
We demonstrate efficient four-wave mixing in low-pressure molecular deuterium without the need for phase matching. We use two laser fields with opposite circular polarizations to produce a strong excitation of a rovibrational transition at a frequency of 3167 cm(-1) . The coherent molecular motion, in turn, modulates a third laser field (also circularly polarized) and results in highly efficient single-sideband conversion.
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