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Advances in Nanoscale Infrared Spectroscopy to Explore Multiphase Polymeric Systems
Published on: June 23, 2023
Local excitation and interference of surface phonon polaritons studied by near-field infrared microscopy
A J Huber1, N Ocelic, R Hillenbrand
1Nano-Photonics Group, Max-Plack-Institut für Biochemie & Center for Nanoscience, München, Germany.
Abstract:
We demonstrate that mid-infrared surface phonon polariton excitation, propagation and interference can be studied by scattering-type near-field optical microscopy (s-SNOM). In our experiments we image surface phonon polaritons (SPPs) propagating on flat SiC crystals. They are excited by weakly focused illumination of single or closely spaced metal disks we fabricated on the SiC surface by conventional photolithography. SPP imaging is performed by pseudo-heterodyne interferometric detection of infrared light scattered by the metal tip of our s-SNOM. The pseudo-heterodyne technique simultaneously yields optical amplitude and phase images which allows us to measure the SPP wave vector--including its sign--and the propagation length and further to study SPP interference. High resolution imaging of SPPs could be applied to investigate for example SPP focusing or heat transfer by SPPs in low dimensional nanostructures.
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