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Updated: Jul 5, 2026

Direct Imaging of Laser-driven Ultrafast Molecular Rotation
Published on: February 4, 2017
Nonintrusive phase stabilization of sub-two-cycle pulses from a prismless octave-spanning Ti:sapphire laser
H M Crespo1, J R Birge, E L Falcão-Filho
1Department of Electrical Engineering and Computer Science and Research Laboratory of Electronics, Massachusetts Institute of Technology, Cambridge, Massachusetts 02139-4307, USA.
Abstract:
Carrier-envelope (CE) phase-stabilized sub-two-cycle pulses are generated from a 500 MHz compact prismless octave-spanning laser without extracavity nonlinear optical processes distorting the laser output. The necessary f and 2f spectral components are generated intracavity and coupled out independently from the main pulse through specially designed cavity mirrors, resulting in a 55 dB CE beat note (100 kHz resolution bandwidth). The in-loop CE phase error (integrated from 2.5 mHz to 10 MHz) is 67 mrad, equivalent to a timing jitter between carrier and envelope of 28 as at 790 nm.

