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From a Natural Product to Its Biosynthetic Gene Cluster: A Demonstration Using Polyketomycin from Streptomyces diastatochromogenes Tü6028
Published on: January 13, 2017
1Department of Chemistry, Metcalf Center for Science and Engineering, Boston University, 590 Commonwealth Avenue, Boston, Massachusetts 02215, USA.
This study presents a new enantioselective synthesis of (-)-kendomycin using an organosilane-based [4 + 2]-annulation strategy. An efficient samarium(II) iodide-assisted cyclization yields the protected macrocycle.
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