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Generation and Coherent Control of Pulsed Quantum Frequency Combs
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Quantum coherent control for nonlinear spectroscopy and microscopy.

Yaron Silberberg1

  • 1Department of Physics of Complex Systems, Weizmann Institute of Science, Rehovot 76100, Israel. yaron.silberberg@weizmann.ac.il

Annual Review of Physical Chemistry
|November 13, 2008
PubMed
Summary
This summary is machine-generated.

Quantum coherent control uses femtosecond pulses to enhance resolution and detection in nonlinear spectroscopy. Applications include improving two-photon absorption and Raman scattering for microscopy and remote sensing.

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Area of Science:

  • Quantum coherent control
  • Atomic and molecular spectroscopy
  • Nonlinear spectroscopy

Background:

  • Quantum coherent control was developed to manipulate molecular systems.
  • Recent advances have expanded its use into atomic and molecular spectroscopy.
  • Femtosecond laser pulses are key tools in this field.

Purpose of the Study:

  • To review the application of femtosecond pulses in nonlinear spectroscopy.
  • To demonstrate enhanced resolution and detection using designed laser pulses.
  • To discuss principles and applications of quantum coherent control.

Main Methods:

  • Utilizing carefully designed femtosecond laser pulses.
  • Investigating two-photon absorption processes.
  • Analyzing coherent anti-Stokes Raman scattering (CARS).

Main Results:

  • Femtosecond pulses can significantly enhance resolution in nonlinear spectroscopy.
  • Improved detection sensitivity is achievable through quantum coherent control.
  • Two-photon absorption and CARS are key areas benefiting from these techniques.

Conclusions:

  • Quantum coherent control with femtosecond pulses offers powerful tools for spectroscopy.
  • Enhanced spectroscopic techniques have potential applications in microscopy and remote sensing.
  • Further development in pulse design can unlock new capabilities.