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Total synthesis of FR901483
Cheryl A Carson1, Michael A Kerr
1Department of Chemistry, The University of Western Ontario, London, Ontario, Canada N6A 5B7.
Organic Letters
|January 14, 2009
Abstract:
The architecturally sophisticated skeleton of the immunosuppressive alkaloid FR901483 was assembled via a process relying on the reaction of an in situ generated imine with a suitably disposed donor-acceptor cyclopropane. A short sequence of functional group transformations provided the natural product in an efficient manner.
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