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Updated: Jun 26, 2026

Ultrafast Time-resolved Near-IR Stimulated Raman Measurements of Functional π-conjugate Systems
Published on: February 10, 2020
All-solid-state parametric Raman anti-Stokes laser at 508 nm.
R P Mildren1, D W Coutts, D J Spence
1MQ Photonics Research Centre, Department of Physics, Macquarie University, NSW 2109, Australia. rmildren@ics.mq.edu.au
Researchers developed a compact parametric anti-Stokes Raman laser using potassium gadolinium tungstate. This laser generates visible light output, demonstrating potential for efficient light generation and wavelength conversion applications.
Area of Science:
- Optics and Photonics
- Laser Physics
- Materials Science
Background:
- Parametric Raman lasers offer tunable wavelength generation.
- Potassium gadolinium tungstate (KGW) is a promising material for nonlinear optical applications.
- Anti-Stokes Raman scattering enables shorter wavelength generation than the pump source.
Purpose of the Study:
- To demonstrate a compact parametric anti-Stokes Raman laser.
- To investigate the performance of potassium gadolinium tungstate in this configuration.
- To achieve efficient generation of visible anti-Stokes light.
Main Methods:
- Utilized a Q-switched 532 nm laser as the pump source.
- Employed a compact 4.5 cm potassium gadolinium tungstate crystal.
- Incorporated an off-axis Stokes resonator for non-collinear phase matching.
Main Results:
- Generated output chiefly at the first anti-Stokes line at 508 nm.
- Achieved anti-Stokes output energies up to 0.27 mJ.
- Observed a pump conversion efficiency of 0.46% for the first anti-Stokes line.
- Detected second- and third-order anti-Stokes lines at 486 nm and 465 nm.
Conclusions:
- The potassium gadolinium tungstate parametric anti-Stokes Raman laser is a compact and efficient device.
- The off-axis resonator design facilitates non-collinear phase matching for anti-Stokes generation.
- The observed multiple anti-Stokes lines suggest potential for broadband visible light generation.
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