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Measurement of Ultrafast Vibrational Coherences in Polyatomic Radical Cations with Strong-Field Adiabatic Ionization
Published on: August 6, 2018
High-order above-threshold ionization with few-cycle pulse: a meter of the absolute phase
Optics Express
|May 26, 2009
Summary
High-order above-threshold ionization reveals an asymmetry in electron emission spectra. This finding allows for the determination of the absolute phase in laser-matter interactions.
Area of Science:
- Quantum Optics
- Atomic, Molecular, and Optical Physics
- Strong Field Physics
Background:
- Above-threshold ionization (ATI) is a fundamental process in strong field physics.
- Understanding the carrier-envelope phase (CEP) dependence of ATI is crucial for controlling electron dynamics.
- Previous studies have explored CEP effects, but detailed analysis of angle-resolved spectra is ongoing.
Purpose of the Study:
- To theoretically investigate angle-resolved energy spectra of high-order ATI.
- To analyze the influence of the carrier-envelope phase (CEP) on these spectra.
- To explore the potential for determining the absolute phase from experimental measurements.
Main Methods:
- Numerical calculation of angle-resolved energy spectra for high-order ATI.
- Simulation using a linearly polarized four-cycle laser pulse.
- Analysis of spectra as a function of the carrier-envelope relative phase (absolute phase).
Main Results:
- Calculated spectra exhibit a distinct left-right (backward-forward) asymmetry.
- This asymmetry is directly correlated with the absolute phase of the laser pulse.
- High-energy electron emission occurs in ultrashort bursts (<0.7 fs), revealing spectral peak structures.
Conclusions:
- The observed spectral asymmetry provides a reliable method for determining the absolute phase in experiments.
- Analysis of peak structures in the spectra offers insights into the time-domain electron emission dynamics.
- These findings advance the understanding and control of electron dynamics in strong laser fields.
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