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Updated: Jun 20, 2026

Multiplex Chemical Imaging Based on Broadband Stimulated Raman Scattering Microscopy
Published on: July 25, 2022
Pump-induced population changes in broadband coherent anti-Stokes Raman scattering
A Gierulski1, M Noda, T Yamamoto
1Nagasaki Research and Development Center, Mitsubishi Heavy Industries, Ltd., 1-2, Akunoura-machi, 850-91 Nagasaki, Japan.
Abstract:
Using a powerful, excimer-laser-pumped broadband coherent anti-Stokes Raman scattering (CARS) system, we have observed considerable changes in the populations of room-temperature nitrogen under atmospheric pressure. Pump-induced populations in the first, second, and third vibronic bands of N2 at room temperature resulted in an apparent vibrational temperature of 2550 K. The implications for broadband N2 CARS thermometry are discussed.
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