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Updated: Jun 19, 2026

Dielectric RheoSANS — Simultaneous Interrogation of Impedance, Rheology and Small Angle Neutron Scattering of Complex Fluids
Published on: April 10, 2017
Observation of a microscopic cascaded contribution to the fifth-order nonlinear susceptibility
Ksenia Dolgaleva1, Heedeuk Shin, Robert W Boyd
1The Institute of Optics, University of Rochester, Rochester, New York 14627, USA. ksenia.dolgaleva@utoronto.ca
Abstract:
Typically, low-order nonlinearities are much stronger than high-order nonlinearities. In this Letter, we demonstrate a procedure by which strong high-order nonlinearities can be synthesized out of low-order nonlinearities. Our procedure involves the use of the previously largely overlooked process of microscopic cascading, which results from local-field effects. We have performed an experiment that allows us to distinguish the influence of microscopic cascading from the more-well-known process of macroscopic cascading, and we find conditions under which microscopic cascading can be the dominant effect. The ability to create a large high-order nonlinear response could prove useful for applications in quantum-information science that require the detection of the simultaneous presence of N entangled photons.
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