Optical sampling by laser cavity tuning
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Updated: Jun 16, 2026

Direct Imaging of Laser-driven Ultrafast Molecular Rotation
Published on: February 4, 2017
Thomas Hochrein1, Rafal Wilk, Michael Mei
1Sueddeutsches Kunststoff-Zentrum, Friedrich-Bergius-Ring 22, Wuerzburg, Germany. T.Hochrein@skz.de
Abstract:
Most time-resolved optical experiments rely either on external mechanical delay lines or on two synchronized femtosecond lasers to achieve a defined temporal delay between two optical pulses. Here, we present a new method which does not require any external delay lines and uses only a single femtosecond laser. It is based on the cross-correlation of an optical pulse with a subsequent pulse from the same laser. Temporal delay between these two pulses is achieved by varying the repetition rate of the laser. We validate the new scheme by a comparison with a cross-correlation measurement carried out with a conventional mechanical delay line.

