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An Experimental Protocol for Femtosecond NIR/UV - XUV Pump-Probe Experiments with Free-Electron Lasers
Published on: October 23, 2018
Characterization of attosecond XUV pulses utilizing a broadband UV approximately VUV pumping
Jun Chen1, Ryuji Itakura, Takashi Nakajima
1Institute of Advanced Energy, Kyoto University, Gokasho, Uji, Kyoto 611-0011, Japan.
Abstract:
We propose a simple scheme to characterize attosecond extreme ultraviolet (XUV) pulses. A broadband ultraviolet (UV) approximately vacuum ultraviolet (VUV) pump pulse creates a coherent superposition of atomic bound states, from which photoionization takes place by the time-delayed attosecond XUV probe pulse. Information on the spectral phase of the XUV pulse can be extracted from the phase offset of the interference beating in the photoelectron spectra using a standard SPIDER (spectral phase interferometry for direct electric-field reconstruction) algorithm. We further discuss the influence of the chirp and polychromaticity of the pump pulse, and show that they do not spoil the reconstruction process. Since our scheme is applicable for various simple atoms such as H, He, and Cs, etc., and capable of characterizing attosecond XUV pulses with a pulse duration of a few hundred attoseconds or even less, it can be an alternative technique to characterize attosecond XUV pulses. Specific numerical examples are presented for the H atom utilizing the 2p and 3p states.
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