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Updated: Jun 15, 2026

Infrared Degenerate Four-wave Mixing with Upconversion Detection for Quantitative Gas Sensing
Published on: March 22, 2019
Single-shot detection and direct control of carrier phase drift of midinfrared pulses
Cristian Manzoni1, Michael Först, Henri Ehrke
1Max Planck Research Group for Structural Dynamics, University of Hamburg, Center for Free Electron Laser Science, c/o DESY, Notkestrasse, 85-22607 Hamburg, Germany. cristian.manzoni@mpsd.cfel.de
Abstract:
We introduce a scheme for single-shot detection and correction of the carrier-envelope phase (CEP) drift of femtosecond pulses at mid-IR wavelengths. Difference frequency mixing between the mid-IR field and a near-IR gate pulse generates a near-IR frequency-shifted pulse, which is then spectrally interfered with a replica of the gate pulse. The spectral interference pattern contains shot-to-shot information of the CEP of the mid-IR field, and it can be used for simultaneous correction of its slow drifts. We apply this technique to detect and compensate long-term phase drifts at 17 microm wavelength, reducing fluctuations to only 110 mrad over hours of operation.
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