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Enhanced sequential carrier capture into individual quantum dots and quantum posts controlled by surface acoustic

Stefan Völk1, Florian J R Schülein, Florian Knall

  • 1Lehrstuhl für Experimentalphysik 1, Universität Augsburg, Universitätsstrasse 1, 86159 Augsburg, Germany.

Nano Letters
|August 21, 2010
PubMed
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Surface acoustic waves switch exciton occupancy in quantum nanostructures. Quantum posts show efficient switching, while quantum dots exhibit hysteresis due to carrier trapping in wetting layers.

Area of Science:

  • * Condensed matter physics
  • * Nanophotonics
  • * Materials science

Background:

  • * Self-assembled quantum dots (QDs) and quantum posts are crucial nanostructures for optoelectronic applications.
  • * Understanding carrier dynamics under external stimuli is key to device optimization.
  • * Surface acoustic waves (SAWs) offer a tunable method to manipulate charge carriers in nanomaterials.

Purpose of the Study:

  • * To investigate the effect of surface acoustic waves (SAWs) on the exciton occupancy of individual quantum dots and quantum posts.
  • * To explore the mechanisms behind acoustically induced switching of charged and neutral excitons.
  • * To compare the SAW response of quantum dots and quantum posts, identifying advantages for specific applications.

Main Methods:

  • * Optical spectroscopy experiments were conducted on individual self-assembled quantum dots and quantum posts.

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  • * The influence of varying surface acoustic wave amplitudes on nanostructure emission was analyzed.
  • * Exciton emission intensity and occupancy switching were monitored as a function of SAW amplitude and sweep direction.
  • Main Results:

    • * SAWs induce switching of exciton occupancy and increase overall emission intensity in both quantum dots and quantum posts.
    • * Quantum posts exhibit continuous switching from charged to neutral excitons, independent of SAW amplitude sweep direction.
    • * Quantum dots display non-monotonic switching with hysteresis, and emission of charged excitons at high SAW amplitudes, attributed to carrier trapping in the wetting layer.

    Conclusions:

    • * Carrier trapping and localization in the wetting layer limit SAW-induced switching in quantum dots.
    • * Quantum posts demonstrate efficient acoustically induced charge transport, overcoming limitations seen in quantum dots.
    • * SAWs provide a viable method for dynamic control of exciton states in quantum nanostructures, with quantum posts showing superior performance.