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Updated: Jun 8, 2026

Measuring Carbon-based Contaminant Mineralization Using Combined CO2 Flux and Radiocarbon Analyses
Published on: October 21, 2016
Regional US carbon sinks from three-dimensional atmospheric CO2 sampling
Cyril Crevoisier1, Colm Sweeney, Manuel Gloor
1Laboratoire de Météorologie Dynamique, Centre National de la Recherche Scientifique, Institut Pierre Simon Laplace, Ecole Polytechnique, 91128 Palaiseau Cedex, France. cyril.crevoisier@lmd.polytechnique.fr
North American carbon budget estimates vary. This study uses atmospheric CO(2) profiles to estimate a moderate land-atmosphere carbon sink for the US, with significant uptake in the Midwest and Southeast.
Area of Science:
- Atmospheric Science
- Ecology
- Climate Science
Background:
- Accurate North American carbon budget quantification is challenging due to data limitations and complex flux modeling.
- Existing studies show substantial divergence on the precise magnitude of the carbon budget.
- Understanding regional carbon fluxes is crucial for climate change mitigation strategies.
Purpose of the Study:
- To estimate land-atmosphere carbon dioxide (CO2) fluxes across North America using a budgeting approach.
- To infer the three-dimensional CO2 distribution over the continent using atmospheric vertical profiles.
- To validate findings against existing carbon cycle reports and identify key regions of carbon uptake.
Main Methods:
- Utilized a simple budgeting approach by balancing tropospheric CO2 inflow and outflow.
- Employed atmospheric CO2 vertical profile data from the National Oceanic and Atmospheric Administration/Earth System Research Laboratory aircraft network.
- Inferred continental-scale CO2 distribution to estimate land-atmosphere fluxes.
Main Results:
- Estimated a moderate sink of 0.5 ± 0.4 Petagrams of Carbon per year (PgC y(-1)) for the coterminous United States during 2004-2006.
- Found good agreement between the estimated sink and the first North American State of the Carbon Cycle Report.
- Identified the Midwest and Southeast as regions with the highest carbon uptake, consistent with crop uptake and forest regrowth estimates.
Conclusions:
- The study provides an independent method for estimating North American carbon budgets.
- Regional carbon uptake is significantly influenced by agricultural activities in the Midwest and forest regrowth in the Southeast.
- Continued atmospheric profile measurements are essential for linking regional carbon uptake to climate drivers.
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