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Updated: Jun 5, 2026

Direct Imaging of Laser-driven Ultrafast Molecular Rotation
Published on: February 4, 2017
Visible laser operation of Pr3+-doped fluoride crystals pumped by a 469 nm blue laser
Bin Xu1, Patrice Camy, Jean-Louis Doualan
1Centre de Recherche sur les Ions, les Matériaux et la Photonique (CIMAP) UMR CEA-CNRS-ENSICaen, Université de Caen, Caen, France.
Abstract:
We report continuous-wave (CW) laser operation of Pr3+-doped LiLuY4, LiYF4 and KY3F10 single crystals in the Red, Orange and Green spectral regions by using a new pumping scheme. The pump source is an especially developed compact, slightly tunable and intracavity frequency-doubled diode-pumped Nd:YAG laser delivering a CW output power of 0.9W at 469.12 nm. At this pump wavelength, efficient room temperature laser emissions corresponding to the 3P0→3F2, 3P0→3H6 and 3P1→3H5 Pr3+ transitions are observed. While a maximum slope efficiency of 45% is obtained in the red with Pr:LiYF4, the demonstration is made for the first time of the orange laser operation of Pr:KY3F10 at about 610 nm.

