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Rational redesign of Candida antarctica lipase B for the ring opening polymerization of D,D-lactide

Mohamad Takwa1, Marianne Wittrup Larsen, Karl Hult

  • 1Royal Institute of Technology, School of Biotechnology, Department of Biochemistry, AlbaNova University Centre, 106 91 Stockholm, Sweden.

Chemical Communications (Cambridge, England)
|May 25, 2011
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Acyclic diene metathesis polymerization or ADMET polymerization involves cross-metathesis of terminal dienes, such as 1,8-nonadiene, to give linear unsaturated polymer and ethylene. As ADMET is a reversible process, the formed ethylene gas must be removed from the reaction mixture to complete the polymerization process.
Similar to cross-metathesis, ADMET also involves the formation of metallacyclobutane intermediate by [2+2] cycloaddition of one of the double bonds of a terminal diene with...