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Single-throughput Complementary High-resolution Analytical Techniques for Characterizing Complex Natural Organic Matter Mixtures
Published on: January 7, 2019
Reduced methane growth rate explained by decreased Northern Hemisphere microbial sources
Fuu Ming Kai1, Stanley C Tyler, James T Randerson
1Department of Earth System Science, University of California, Irvine, California 92697, USA. fmkai@smart.mit.edu
Atmospheric methane (CH4) growth slowed due to reduced Northern Hemisphere microbial sources, particularly from Asian rice agriculture. This finding clarifies the atmospheric methane puzzle around the millennium. Keywords: atmospheric methane, microbial sources, rice agriculture.
Area of Science:
- Atmospheric chemistry and climate science.
- Biogeochemical cycles and greenhouse gas emissions.
Background:
- Atmospheric methane (CH4) levels rose through the 20th century, then slowed before increasing again.
- Previous studies cited fossil fuels, wetlands, agriculture, and hydroxyl (OH) sinks as potential causes for the slowdown.
Purpose of the Study:
- To investigate the primary drivers of the late-twentieth-century slowdown in atmospheric methane growth rates.
- To differentiate contributions from various methane sources and sinks using isotopic analysis.
Main Methods:
- Analysis of synchronous time series of atmospheric CH4 mixing ratios and carbon isotope ratios ((13)C/(12)C).
- Utilized a two-box atmospheric model to simulate CH4 evolution.
- Compared observed isotopic changes with modeled scenarios of source and sink variations.
Main Results:
- Reduced microbial sources in the Northern Hemisphere best explain the observed CH4 growth rate changes.
- Isotopic data exclude reduced fossil fuel emissions as the main cause of the slowdown.
- Northern Hemisphere agricultural emissions, especially from rice cultivation in Asia, account for approximately 51% of the emission decrease, linked to fertilizer use and water management.
Conclusions:
- The late-20th century atmospheric methane slowdown was primarily driven by decreased microbial emissions in the Northern Hemisphere.
- Changes in Asian rice agriculture significantly contributed to this reduction.
- Further research into microbial methane sources and agricultural practices is warranted.
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