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Effect of specimen misalignment on local structure analysis using annular dark-field imaging.

Yeong-Gi So1, Koji Kimoto

  • 1National Institute for Materials Science, 1-1 Namiki, Tsukuba, Ibaraki 305-0044, Japan. so.yeonggi@nims.go.jp

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Crystal tilt in scanning transmission electron microscopy (STEM) with annular dark-field (ADF) imaging causes artifacts. Using a large convergence angle improves atomic position accuracy and spatial resolution by minimizing these imaging errors.

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Area of Science:

  • Materials Science
  • Physics
  • Electron Microscopy

Background:

  • Annular dark-field (ADF) imaging in scanning transmission electron microscopy (STEM) is crucial for atomic resolution.
  • Crystal tilt, a slight misalignment, can introduce artifacts in STEM-ADF images, complicating analysis.

Purpose of the Study:

  • To investigate the impact of crystal tilt on ADF imaging in STEM.
  • To determine how probe convergence angle affects image fidelity and artifact formation.

Main Methods:

  • Simulated STEM-ADF imaging under varying crystal tilt conditions.
  • Analysis of image artifacts, specifically spot displacements, for different convergence angles.
  • Utilized multislice simulation to model electron scattering and image formation.

Main Results:

  • Small convergence angles in STEM-ADF imaging lead to spot shifts and breakdown of the incoherent imaging approximation due to crystal tilt.
  • Large convergence angles result in bright spot positions accurately reflecting atomic column positions.
  • Multislice simulations revealed that a smaller depth of focus at large convergence angles enhances interpretability.

Conclusions:

  • A large convergence angle in STEM-ADF imaging mitigates crystal tilt artifacts.
  • This approach enables more accurate measurement of atomic positions.
  • Improved spatial resolution and reliable atomic site determination are achieved with larger convergence angles.