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Updated: May 20, 2026

High Resolution Phonon-assisted Quasi-resonance Fluorescence Spectroscopy
Published on: June 28, 2016
Enhancement of spectral resolution and accuracy in asynchronous-optical-sampling terahertz time-domain spectroscopy
Takeshi Yasui1, Kohji Kawamoto, Yi-Da Hsieh
1Graduate School of Engineering Science, Osaka University, 1-3 Machikaneyama, Toyonaka, Osaka 560-8531, Japan. yasui@me.tokushima-u.ac.jp
Abstract:
The spectral resolution and accuracy of asynchronous-optical-sampling terahertz time-domain spectroscopy (ASOPS-THz-TDS) were evaluated by examining low-pressure gas-phase samples. Use of dual 56-MHz, erbium (Er)-doped, mode-locked femtosecond fiber lasers enhanced the spectral resolution to as low as 50.5 MHz and the spectral accuracy to as low as 6.2 × 10(-6). The results indicate that ASOPS-THz-TDS has the potential to achieve high spectral resolution, high spectral accuracy, and wide spectral coverage at the same time. ASOPS-THz-TDS will open a new door to gas-phase spectroscopy of multiple chemical species in the field of atmospheric gas analysis.

