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Published on: July 17, 2019
Substrate coupling suppresses size dependence of thermal conductivity in supported graphene
Jie Chen1, Gang Zhang, Baowen Li
1Department of Physics, Centre for Computational Science and Engineering, National University of Singapore, Singapore 117542. phychenj@nus.edu.sg
Abstract:
Thermal conductivity κ of both suspended and supported graphene has been studied by using molecular dynamics simulations. An obvious length dependence is observed in κ of suspended single-layer graphene (SLG), while κ of supported SLG is insensitive to the length. The simulation result of room temperature κ of supported SLG is in good agreement with the experimental value. In contrast to the decrease in κ induced by inter-layer interaction in suspended few-layer graphene (FLG), κ of supported FLG is found to increase rapidly with the layer thickness, reaching about 90% of that of bulk graphite at six layers, and eventually saturates at the thickness of 13.4 nm. More interestingly, unlike the remarkable substrate dependent κ in SLG, the effect of substrate on thermal transport is much weaker in FLG. The underlying physics is investigated and presented.
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