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Updated: May 9, 2026

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An Experimental Protocol for Femtosecond NIR/UV - XUV Pump-Probe Experiments with Free-Electron Lasers
Published on: October 23, 2018
Zeptosecond high harmonic keV x-ray waveforms driven by midinfrared laser pulses
C Hernández-García1, J A Pérez-Hernández, T Popmintchev
1Grupo de Investigación en Óptica Extrema, Universidad de Salamanca, E-37008 Salamanca, Spain. carloshergar@usal.es
Physical Review Letters
|August 6, 2013
Summary
Mid-infrared lasers produce high harmonic X-ray pulses with unique zeptosecond structures, unlike near-infrared lasers. This temporal fine structure in X-ray generation allows for the creation of sub-attosecond waveforms.
Area of Science:
- Quantum optics
- Attosecond science
- Laser-driven phenomena
Background:
- High harmonic generation (HHG) is a key process for producing extreme ultraviolet (XUV) and X-ray light.
- The temporal characteristics of HHG pulses are crucial for ultrafast science applications.
- The choice of laser driver (e.g., near-infrared vs. mid-infrared) can significantly impact the generated X-ray properties.
Purpose of the Study:
- To theoretically investigate the temporal structure of high harmonic X-ray pulses generated by mid-infrared lasers.
- To compare the temporal characteristics of X-ray pulses generated by mid-infrared and near-infrared lasers.
- To explore the potential for generating sub-attosecond X-ray waveforms.
Main Methods:
- Theoretical modeling of high harmonic generation.
- Simulation of electron wave packet dynamics and reencounters with the ion.
- Analysis of the interference effects in high harmonic emission.
Main Results:
- Mid-infrared lasers produce X-ray pulses with distinct temporal structures compared to near-infrared lasers, particularly at high photon energies.
- The femtosecond-scale X-ray bursts exhibit an intrinsic zeptosecond substructure due to multi-electron reencounter interference.
- Regular sub-attosecond X-ray waveforms can be generated by appropriate filtering without chirp compensation.
Conclusions:
- The temporal fine structure of X-ray pulses is highly dependent on the driving laser's infrared wavelength.
- Zeptosecond structuring in high harmonic generation opens new avenues for attosecond X-ray waveform control.
- This work provides a theoretical basis for generating attosecond X-ray pulses for advanced scientific investigations.

