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Onsager's Wien effect on a lattice.

V Kaiser1, S T Bramwell, P C W Holdsworth

  • 11] Max-Planck-Institut für Physik komplexer Systeme, Nöthnitzer Straße 38, 01187 Dresden, Germany [2] Université de Lyon, Laboratoire de Physique, École Normale Supérieure de Lyon, 46 allée d'Italie, 69364 Lyon CEDEX 07, France.

Nature Materials
|August 13, 2013
PubMed
Summary
This summary is machine-generated.

Simulations of the second Wien effect in electrolytes confirm Onsager theory, revealing how microscopic dynamics influence conductivity. Lattice simulations offer a powerful tool for studying this phenomenon in diverse applications.

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Area of Science:

  • Physical Chemistry
  • Computational Physics

Background:

  • The second Wien effect describes electrolyte response to electric fields, crucial for applications like solar cells and semiconductors.
  • Onsager's electrodiffusion theory (1934) explains this effect but lacks numerical simulation validation.

Discussion:

  • This study presents the first numerical simulations of the second Wien effect using a lattice Coulomb gas model.
  • The simulations focus on systems with double equilibrium for free charge generation.

Key Insights:

  • Simulations confirm Onsager's theory regarding field evolution of charge density and correlations.
  • Numerical methods reveal corrections to conductivity influenced by microscopic dynamics, going beyond analytical predictions.

Outlook:

  • Lattice simulations provide a versatile tool for investigating system-specific corrections to Onsager's theory.
  • This approach aids in understanding the practical applications of the second Wien effect in various scientific and technological fields.