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Dynamic competition between spin-density wave order and superconductivity in underdoped Ba(1-x)K(x)Fe2As2
11] Stanford Institute for Materials and Energy Sciences, SLAC National Accelerator Laboratory and Stanford University, Menlo Park, California 94025, USA [2] Departments of Physics and Applied Physics, and Geballe Laboratory for Advanced Materials, Stanford University, Stanford, California 94305, USA.
In iron pnictides, superconductivity competes with spin-density wave (SDW) and nematic orders. This study shows both SDW and superconducting gaps coexist, with the SDW gap shrinking as superconductivity emerges.
Area of Science:
- Condensed Matter Physics
- Materials Science
- Quantum Materials
Background:
- Unconventional superconductivity often emerges near competing electronic phases.
- Iron pnictides exhibit competing tetragonal-to-orthorhombic structural and spin-density wave (SDW) transitions near superconductivity.
- Macroscopic evidence suggests competition, with suppressed orthorhombicity and magnetic moments in superconducting states.
Purpose of the Study:
- To spectroscopically investigate the coexistence and competition between superconductivity, SDW order, and electronic nematicity in iron pnictides.
- To provide direct evidence for the dynamic interplay of these phases at the electronic level.
Main Methods:
- Angle-resolved photoemission spectroscopy (ARPES) was performed on detwinned, underdoped Ba(1-x)K(x)Fe2As2 samples.
- ARPES allowed for the visualization of electronic band structures and energy gaps.
Main Results:
- Direct observation of the coexistence of both a spin-density wave (SDW) gap and a superconducting gap within the same electronic structure.
- Following the onset of superconductivity, a decrease in the magnitude of the SDW gap was detected.
- The SDW gap's shift indicated a reduction in orbital anisotropy, consistent with nematic order suppression.
Conclusions:
- The study provides direct spectroscopic evidence for the dynamic competition between superconductivity, SDW order, and electronic nematicity in iron pnictides.
- Suppression of competing orders is crucial for the emergence and behavior of superconductivity in these materials.
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