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Determination of the Excitation and Coupling Rates Between Light Emitters and Surface Plasmon Polaritons
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Percolating plasmonic networks for light emission control.

Michele Gaio1, Marta Castro-Lopez, Jan Renger

  • 1Department of Physics, King's College London, Strand, London WCR 2LS, UK. michele.gaio@kcl.ac.uk riccardo.sapienza@kcl.ac.uk.

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Summary
This summary is machine-generated.

Local electromagnetic fields in plasmonic nanoantennas significantly influence light emission. These nanoantennas, featuring fractal gold networks near percolation, show that local properties dominate fluorescence modification, not long-range interactions.

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Area of Science:

  • Nanophotonics
  • Plasmonics
  • Materials Science

Background:

  • Optical nanoantennas enable precise manipulation of single photons in nanostructured environments.
  • Complex plasmonic architectures offer multiscale control over light wavelength and mode matching.

Purpose of the Study:

  • Investigate the impact of plasmonic network formation on light emission from embedded fluorescent probes.
  • Analyze the interplay between global and local optical properties in self-assembled and lithographic gold films.

Main Methods:

  • Fabrication and characterization of self-assembled semi-continuous gold films and lithographic gold networks.
  • Fluorescence dynamics experiments to probe light-matter interactions.
  • Analysis of local density of optical states (LDOS) fluctuations near the electrical percolation threshold.

Main Results:

  • Plasmonic networks exhibit large LDOS fluctuations around the percolation threshold, characterized by fractal topology.
  • Both global long-range interactions (percolation, fractality) and local near-field effects influence fluorescence.
  • Local electromagnetic field contributions and network topology were found to be the dominant factors in fluorescence modification.

Conclusions:

  • Local optical properties of plasmonic nanoantennas play a critical role in modifying light emission.
  • The fractal topology and electrical percolation of gold networks significantly impact plasmonic behavior.
  • Understanding local near-field effects is key for designing advanced nanophotonic devices.