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Updated: Jan 4, 2026

Measurement of Ultrafast Vibrational Coherences in Polyatomic Radical Cations with Strong-Field Adiabatic Ionization
Published on: August 6, 2018
Tunneling dynamics in multiphoton ionization and attoclock calibration.
Michael Klaiber1, Karen Z Hatsagortsyan1, Christoph H Keitel1
1Max-Planck-Institut für Kernphysik, Saupfercheckweg 1, 69117 Heidelberg, Germany.
Investigating strong-field ionization, this study reveals nonadiabatic effects that alter electron trajectories and modify Coulomb focusing. These findings offer insights into tunneling dynamics and attoclock calibration.
Area of Science:
- Atomic, Molecular, and Optical Physics
- Quantum Dynamics
- Strong-Field Physics
Background:
- Strong-field ionization is crucial for understanding electron dynamics in intense laser fields.
- The intermediate domain between tunneling and multiphoton ionization presents complex electron behavior.
- Accurate modeling is needed to interpret experimental results, such as those from the attoclock technique.
Purpose of the Study:
- To investigate the intermediate domain of strong-field ionization.
- To develop an intuitive model for ionization dynamics incorporating nonadiabatic effects.
- To explore the influence of these effects on electron wave packet behavior and Coulomb focusing.
Main Methods:
- Utilizing the strong-field approximation (SFA).
- Employing the imaginary-time method for theoretical analysis.
- Developing a nonadiabatic tunneling model with coordinate-dependent electron energy.
Main Results:
- Nonadiabatic effects induce transversal momentum shifts and delayed electron appearance.
- The tunneling exit shifts towards the ionic core, significantly altering Coulomb focusing.
- Including the Coulomb field during under-the-barrier motion amplifies nonadiabatic effects.
Conclusions:
- The modified simple man model provides an intuitive framework for understanding complex ionization dynamics.
- Nonadiabatic corrections are essential for accurate descriptions of electron behavior in strong laser fields.
- The findings have direct implications for calibrating and interpreting attoclock measurements.
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