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Ultrafast Dynamics of Lasing Semiconductor Nanowires.

Robert Röder1, Themistoklis P H Sidiropoulos2, Christian Tessarek3,4

  • 1†Institute of Solid State Physics, Friedrich-Schiller-University Jena, Max-Wien-Platz 1, 07743 Jena, Germany.

Nano Letters
|June 19, 2015
PubMed
Summary
This summary is machine-generated.

Ultrafast semiconductor nanowire lasers exhibit picosecond onset times, influenced by material properties and excitation wavelength. Pulse width depends on nanowire diameter, indicating a transition in waveguiding modes.

Keywords:
Semiconductor nanowirecarrier thermalizationcarrier−phonon interactiononset timepulse widthultrafast lasing

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Area of Science:

  • Optoelectronics
  • Materials Science
  • Nanotechnology

Background:

  • Semiconductor nanowire lasers are crucial for ultrafast optical applications.
  • Understanding their temporal dynamics, such as laser onset and pulse width, is essential for device optimization.

Purpose of the Study:

  • To investigate the temporal dynamics of semiconductor nanowire lasers, specifically laser onset time and pulse width.
  • To explore the influence of material properties, excitation wavelength, and nanowire dimensions on these dynamics.

Main Methods:

  • Employed a double-pump approach to measure temporal dynamics.
  • Studied wide bandgap materials: gallium nitride (GaN), zinc oxide (ZnO), and cadmium sulfide (CdS) nanowires.
  • Analyzed the effect of varying nanowire sizes and excitation wavelengths.

Main Results:

  • Laser onset times were found to be in the picosecond range, driven by carrier thermalization.
  • ZnO exhibited the fastest onset time (~1 ps) due to strong carrier-phonon coupling, followed by CdS (~2.5 ps) and GaN (~3.5 ps).
  • Onset times were independent of nanowire size but varied with excitation wavelength relative to the band gap.
  • Pulse widths depended on the optical system, with a critical diameter transition from ~5 ps to ~15 ps observed, linked to single-to-multimode waveguiding.

Conclusions:

  • Carrier thermalization dictates the picosecond laser onset in semiconductor nanowires.
  • Material-specific carrier-phonon coupling significantly impacts laser dynamics.
  • Nanowire diameter plays a critical role in pulse width by influencing waveguiding modes.