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Dynamical Fano-Like Interference between Rabi Oscillations and Coherent Phonons in a Semiconductor Microcavity

S Yoshino1, G Oohata1, K Mizoguchi1

  • 1Department of Physical Science, Graduate School of Science, Osaka Prefecture University, 1-1 Gakuen-cho, Naka-ku, Sakai 599-8531, Japan.

Physical Review Letters
|November 10, 2015
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Summary
This summary is machine-generated.

We observed dynamical interference between Rabi oscillations and coherent phonons in CuCl semiconductor microcavities. This coupling enhances phonon intensity and creates asymmetric spectral structures due to constructive and destructive interference.

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Area of Science:

  • Condensed Matter Physics
  • Semiconductor Optics
  • Quantum Dynamics

Background:

  • Semiconductor microcavities exhibit complex light-matter interactions.
  • Coherent phonons and Rabi oscillations are key phenomena in ultrafast spectroscopy.
  • Understanding their interplay is crucial for advanced optical devices.

Purpose of the Study:

  • To investigate the dynamical interference between Rabi oscillations and coherent phonons in CuCl.
  • To elucidate the coupling mechanisms and their impact on spectral properties.
  • To model the observed interference phenomena.

Main Methods:

  • Time-domain pump-probe spectroscopy on CuCl semiconductor microcavities.
  • Fourier transformation of time-domain signals.
  • Continuous wavelet transformation for time-frequency analysis.
  • Classical coupled oscillator modeling.

Main Results:

  • Rabi oscillations were found to drive coherent longitudinal optical phonons in CuCl via Fröhlich interaction.
  • Phonon intensity increased with Rabi oscillation intensity.
  • Spectral profiles of coherent phonons shifted from peak to dip with asymmetric structures upon frequency detuning.
  • Interference patterns were attributed to constructive and destructive interference between oscillations and phonons.

Conclusions:

  • Dynamical Fano-like interference governs the interaction between Rabi oscillations and coherent phonons.
  • A classical coupled oscillator model accurately reproduces the observed asymmetric spectral structures.
  • This study provides insights into controlling phonon behavior through light-matter coupling in semiconductors.