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Rational design and synthesis of a porous, task-specific polycarbazole for efficient CO2 capture
Tian Jin1, Yan Xiong1, Xiang Zhu2
1State Key Laboratory of Chemical Engineering and Department of Chemistry, East China University of Science and Technology, Shanghai, 200237, P. R. China. hlliu@ecust.edu.cn.
Chemical Communications (Cambridge, England)
|February 12, 2016
Abstract:
We present a rational design and synthesis of a novel porous pyridine-functionalized polycarbazole for efficient CO2 capture based on the density functional theory calculations. The task-specific polymer, generated through a one-step FeCl3-catalyzed oxidative coupling reaction, exhibits a superior CO2 uptake at 1.0 bar and 273 K (5.57 mmol g(-1)).
