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Updated: Mar 21, 2026

An Experimental Protocol for Femtosecond NIR/UV - XUV Pump-Probe Experiments with Free-Electron Lasers
Published on: October 23, 2018
Wavelength-tunable split-and-delay optical system for hard X-ray free-electron lasers.
Researchers developed a hard X-ray split-and-delay optical (SDO) system for precise temporal separation of X-ray pulses. This advancement enables new time-resolved studies at X-ray free-electron laser facilities.
Area of Science:
- Optics and photonics
- Materials science
- X-ray physics
Background:
- Generating precisely timed X-ray pulses is crucial for advanced scientific research.
- Existing methods for temporal separation of X-ray pulses have limitations in stability and flexibility.
Purpose of the Study:
- To develop a stable and flexible hard X-ray split-and-delay optical (SDO) system.
- To enable variable temporal separation of X-ray pulses for time-resolved studies.
Main Methods:
- Designed an SDO system with variable-delay and fixed-delay branches.
- Fabricated high-quality thin and channel-cut crystals using plasma chemical vaporization machining.
- Developed a simple alignment method for spatial overlap of split pulses.
Main Results:
- The SDO system achieved a wide photon energy range (6.5-11.5 keV) and extensive delay times (up to 220 ps).
- Excellent spatial overlap of split pulses (30 nm accuracy) was demonstrated for focused beams.
- The system demonstrated high stability and operational flexibility.
Conclusions:
- The developed hard X-ray SDO system is a significant advancement for time-resolved X-ray studies.
- This technology facilitates femtosecond to subnanosecond time-resolved experiments at X-ray free-electron laser facilities.
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