First study on ²³⁶U in the Northeast Pacific Ocean using a new target preparation procedure for AMS measurements

We succeeded in obtaining the depth profile of ²³⁶U for a sampling station in the Northeast Pacific Ocean using only one litre of seawater sample from each depth. For this purpose, a new procedure was developed that allowed for the preparation of accelerator mass spectrometry targets for trace uranium using only 100 μg of iron carrier material. The ²³⁶U concentrations in water samples from the Northeast Pacific Ocean showed large variations from (9.26 ± 0.42) × 10⁶ atoms/kg at 60 m depth to (0.08 ± 0.02) × 10⁶ atoms/kg at a depth of 3000 m. The high ²³⁶U concentrations in surface water reflect the input of ²³⁶U by global and local fallout from nuclear weapons tests. The low ²³⁶U concentrations in seawater from 1500 m and below are an indicator for the low vertical diffusion of surface water to deeper layers in the North Pacific Ocean. The total inventory of ²³⁶U on the water column was (8.35 ± 0.23) × 10¹² atoms/m², which is lower compared to those of other ocean regions solely affected by global fallout on comparable latitudes. This study represents the first dataset for ²³⁶U in the Pacific Ocean and shows the possibility of downsizing sample volumes which may help in future applications of ²³⁶U as tracer for large ocean areas.