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Zinc-Sponge Battery Electrodes that Suppress Dendrites
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Suppressing Lithium Dendrite Growth with a Single-Component Coating.

Haodong Liu1, Hongyao Zhou1, Byoung-Sun Lee1

  • 1Department of NanoEngineering, University of California San Diego , La Jolla, California 92093, United States.

ACS Applied Materials & Interfaces
|August 23, 2017
PubMed
Summary
This summary is machine-generated.

A novel coating on lithium metal, formed from lithium iodide and organic carbonates, prevents dendrite growth during battery cycling. This stable layer enhances lithium metal battery performance and longevity.

Keywords:
LiIchemically homogeneous coatingdendrite-freelithium methyl carbonatelithium-metal anodesingle-component coating

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Area of Science:

  • Materials Science
  • Electrochemistry
  • Battery Technology

Background:

  • Lithium metal anodes are crucial for high-energy-density batteries.
  • Dendrite formation during lithium cycling leads to capacity fading and safety hazards.
  • Stable solid-electrolyte interphase (SEI) layers are essential for lithium metal battery longevity.

Purpose of the Study:

  • To develop a single-component coating for lithium metal anodes.
  • To investigate the formation mechanism and properties of the coating.
  • To evaluate the performance of the coated lithium metal in battery cycling.

Main Methods:

  • Formation of a coating on lithium metal using lithium iodide in dimethyl carbonate (DMC) and ethylene carbonate (EC) electrolyte.
  • Chemical reaction analysis between lithium iodide and DMC to form lithium methyl carbonate (LMC).
  • Symmetric Li||Li cell testing at a current density of 3 mA cm⁻² to assess cycling stability and dendrite suppression.

Main Results:

  • A chemically homogeneous coating layer of lithium methyl carbonate (LMC) was successfully formed on the lithium metal surface.
  • The LMC coating enabled dendrite-free lithium cycling in a symmetric Li||Li cell at 3 mA cm⁻².
  • Addition of EC to DMC modulated LMC formation, leading to a stable coating crucial for long-term cycling.
  • The coating demonstrated compatibility with standard LiPF₆/carbonate electrolytes used with metal oxide cathodes.

Conclusions:

  • A single-component LMC coating effectively suppresses lithium dendrite growth.
  • The coating enhances the cycling stability and longevity of lithium metal anodes.
  • This protective layer offers a promising strategy for developing safer and more efficient lithium metal batteries.