Moiré Superstructure and Dimensional Crossover of 2D Electronic States on Nanoscale Lead Quantum Films

We investigate using scanning tunneling microscopy and spectroscopy electronic aspects of Moiré superstructures in nanoscale Pb quantum films grown on IrTe₂, which is a unique layered material with charge-order transitions into stripe phases. Pb ultrathin films exhibit a Moiré superstructure due to the lattice mismatch of Pb and IrTe₂, which produces strong lateral electronic modulation of hexagonal symmetry and discreet subbands. Moreover, strongly anisotropic or 1D electronic states are formed in Pb films as modulated by the stripe charge order. Present results indicate the controllability of lateral electronic structures of various ultrathin films by extra interfacial potentials due not only to Moiré superstructures but also to novel electronic orderings of substrates.