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An Experimental Protocol for Femtosecond NIR/UV - XUV Pump-Probe Experiments with Free-Electron Lasers
Published on: October 23, 2018
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THz-pump and X-ray-probe sources based on an electron linac
Sadiq Setiniyaz1, Seong Hee Park2, Hyun Woo Kim1
1Korea Atomic Energy Research Institute, 1045 Daedeok-Daero, Yuseong-gu, Daejeon 34057, South Korea.
The Review of Scientific Instruments
|December 3, 2017
Summary
This study introduces a compact THz-pump and X-ray-probe beamline for ultrafast time-resolved diffraction. The system generates synchronized THz and X-ray pulses using an electron linac, enabling advanced material analysis.
Area of Science:
- Physics
- Materials Science
- Spectroscopy
Background:
- Ultrafast time-resolved diffraction requires synchronized pump-probe capabilities.
- Existing methods may lack the necessary temporal resolution or flux for certain applications.
- Compact, efficient beamlines are crucial for broader accessibility in scientific research.
Purpose of the Study:
- To present a novel, compact THz-pump and X-ray-probe beamline.
- To demonstrate simultaneous generation of THz radiation and hard X-rays from an electron linac.
- To enable high-resolution ultrafast time-resolved diffraction studies.
Main Methods:
- Utilizing a compact electron linac to generate two high-energy electron bunches.
- Employing a multifoil radiator to simultaneously produce THz radiation and hard X-rays.
- Implementing an adjustable optical delay for precise synchronization of THz and X-ray pulses.
- Conducting GEANT4 simulations to optimize radiator design and predict X-ray yield.
Main Results:
- Achieved peak THz power of 0.14 GW from a multifoil radiator with a 200 pC electron bunch.
- Optimized carbon foil radiators (0.5-1.0 mm) for high yield of 10-20 keV hard X-rays (approx. 10^3 photons/(keV pC-electrons)).
- Demonstrated generation of ~10^7 X-rays per 1 keV energy bin per second at 100 Hz repetition rate.
- Observed X-ray pulse durations of 400-600 fs, with minimal radiator heating.
Conclusions:
- The developed beamline offers a compact and efficient solution for ultrafast time-resolved diffraction.
- The synchronized THz and X-ray pulses enable advanced studies of dynamic processes in materials.
- The system's design parameters suggest high potential for various scientific investigations.

