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Updated: Feb 16, 2026

Direct Imaging of Laser-driven Ultrafast Molecular Rotation
Published on: February 4, 2017
Characterization of two ultrashort laser pulses using interferometric imaging of self-diffraction
Abstract:
Noncollinear pulse characterization methods can be applied to over-octave spanning waveforms, but geometrical effects in the nonlinear medium such as beam smearing and critical sensitivity to beam alignment hinder their accurate application. Here, a method is introduced for the temporal and spatial characterization of two pulses by interferometric, spectrally resolved imaging of self-diffraction. Geometrical effects are resolved by the method and, therefore, do not limit the accuracy. Two methods for quantitative pulse retrieval are presented. One method is analytical and very fast; the other method is iterative and more robust if applied to noisy data.

