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All-Solid-State Batteries with Thick Electrode Configurations.

Yuki Kato1,2, Shinya Shiotani2,3, Keisuke Morita2

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Researchers developed thick electrode all-solid-state lithium-ion cells achieving high capacity. They analyzed ionic conductivity and tortuosity effects on performance, providing key insights for advanced battery design.

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Area of Science:

  • Materials Science
  • Electrochemistry
  • Energy Storage

Background:

  • All-solid-state lithium-ion batteries offer enhanced safety and energy density.
  • Thick electrodes are crucial for high-capacity energy storage but present challenges in ion transport.

Purpose of the Study:

  • To prepare and characterize thick electrode all-solid-state lithium-ion cells.
  • To investigate the influence of ionic conductivity and electrode tortuosity on cell performance.

Main Methods:

  • Fabrication of all-solid-state lithium-ion cells with 600 μm-thick cathode layers.
  • Electrochemical testing at room temperature to assess discharge performance.
  • Analysis of capacity-current data to determine the tortuosity factor.

Main Results:

  • Achieved a high geometric capacity of 15.7 mAh cm⁻² at room temperature.
  • Demonstrated the impact of solid electrolyte ionic conductivity on discharge performance.
  • Quantitatively evaluated the tortuosity factor and its effect on cell performance.

Conclusions:

  • Thick electrode designs are viable for high-capacity all-solid-state lithium-ion cells.
  • Electrode tortuosity is a critical parameter influencing electrochemical performance.
  • Understanding these factors is essential for optimizing future battery development.