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Forced Wetting Transition and Bubble Pinch-Off in a Capillary Tube.

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In partial wetting, increasing fluid displacement rates in capillary tubes causes a wetting transition. This phenomenon leads to bubble pinch-off, even without geometric constraints, impacting microfluidic devices.

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Area of Science:

  • Fluid dynamics
  • Surface science
  • Microfluidics

Background:

  • Immiscible fluid displacement in partial wetting presents challenges in both microscopic and macroscopic understanding.
  • Classic fluid displacement models often assume complete wetting, which may not reflect real-world scenarios.

Purpose of the Study:

  • To investigate the fluid-fluid displacement of a viscous fluid by a less viscous fluid in a circular capillary tube under partial wetting conditions.
  • To identify the conditions under which a wetting transition occurs and its impact on interface behavior and bubble formation.

Main Methods:

  • Studied fluid displacement in a circular capillary tube using a less viscous fluid displacing a more viscous one.
  • Analyzed the behavior of the fluid-fluid interface and contact line at varying displacement rates (capillary numbers).
  • Investigated the dewetting of entrained films and subsequent bubble pinch-off dynamics.

Main Results:

  • A contact angle-dependent wetting transition occurs at a critical capillary number.
  • At low rates, the interface moves without shape change; at higher rates, it becomes unstable, forming a finger.
  • An entrained film dewets, universally leading to bubble pinch-off, driven by contact line hydrodynamics.

Conclusions:

  • The study demonstrates that moving contact line hydrodynamics can generate bubbles in microfluidic devices, irrespective of geometric constraints.
  • The findings challenge existing models by showing a dynamic wetting transition in partial wetting regimes.
  • This research provides new insights into fluid behavior in microscale systems relevant to microfluidics and materials science.