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Strand Plasticity Governs Fatigue in Colloidal Gels
Jan Maarten van Doorn1, Joanne E Verweij1, Joris Sprakel1
1Physical Chemistry and Soft Matter, Wageningen University, Stippeneng 4, 6708 WE Wageningen, The Netherlands.
Physical Review Letters
|June 5, 2018
Summary
Microscopic plasticity drives fatigue in soft solids. Irreversible strand stretching causes network softening and strain hardening, revealing new insights into material failure.
Area of Science:
- Materials Science
- Soft Matter Physics
- Rheology
Background:
- Material fatigue, driven by repeated loading, causes catastrophic failure.
- The microscopic origins of fatigue in soft solids are not well understood.
- Colloidal gels serve as model systems for inhomogeneous soft solids.
Purpose of the Study:
- To investigate the microscopic mechanisms of fatigue in colloidal gels.
- To elucidate the relationship between mechanical loading and microstructural changes.
- To develop a new understanding of fatigue in soft thermal solids.
Main Methods:
- Combined experimental techniques with computer simulations.
- Applied repeated mechanical loading to colloidal gel samples.
- Analyzed microstructural evolution and mechanical response at various deformation scales.
Main Results:
- Identified irreversible strand stretching as a key mechanism under mechanical load.
- Observed network softening at small strains due to induced slack.
- Documented strain hardening at larger deformations.
- Demonstrated that microscopic plasticity governs macroscopic fatigue behavior.
Conclusions:
- Microscopic plasticity is the primary driver of fatigue in soft solids.
- Fatigue in soft thermal solids requires new theoretical frameworks incorporating local plasticity.
- This study provides a novel perspective on soft gel mechanics and failure.
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