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Single-Digit Nanometer Electron-Beam Lithography with an Aberration-Corrected Scanning Transmission Electron Microscope
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Magnetic Patterning by Electron Beam-Assisted Carbon Lithography.

Pietro Genoni1, Francesca Genuzio2, Tevfik Onur Menteş2

  • 1CIMAINA, Department of Physics , Università degli Studi di Milano , via Celoria 16 , I-20133 Milan , Italy.

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|July 19, 2018
PubMed
Summary

We developed a scalable method to pattern magnetic states using electron beams to create chemical patterns. This process induces spin reorientation transitions in cobalt, enabling control over magnetic anisotropy in specific regions.

Keywords:
chiral domain wallscobalt thin filmsmagnetic lithographypatterningspin reorientation transition

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Area of Science:

  • Surface Science
  • Materials Science
  • Nanotechnology

Background:

  • Controlling magnetic properties at the nanoscale is crucial for advanced electronic devices.
  • Patterning magnetic materials with high resolution remains a significant challenge.

Purpose of the Study:

  • To demonstrate a scalable method for writing magnetic states on ultrathin cobalt films.
  • To achieve lateral control over magnetic anisotropy using chemical patterning.

Main Methods:

  • Electron-stimulated molecular dissociative adsorption of carbon monoxide on ultrathin Co/Re(0001).
  • Microfocused low-energy electron beams to induce fragmentation and surface carbide/graphitic carbon formation.
  • Annealing to create nanometer-sharp chemical patterns.

Main Results:

  • Carbon accumulation in irradiated areas induces an in-plane to out-of-plane spin reorientation transition in cobalt.
  • Formation of striped magnetic domains and out-of-plane magnetic anisotropy under a graphitic overlayer.
  • Chiral Néel walls separating domains with opposite magnetization.

Conclusions:

  • The developed protocol offers lateral control over spin reorientation transitions.
  • Magnetic anisotropy can be tuned in arbitrary mesoscopic regions.
  • Potential applications in nano-engineering of magnetic stacks and graphene-based devices.