Effect of Sharp Diameter Geometrical Modulation on the Magnetization Reversal of Bi-Segmented FeNi Nanowires

Controlling functional properties of matter and combining them for engineering a functional device is, nowadays, a common direction of the scientific community. For instance, heterogeneous magnetic nanostructures can make use of different types of geometrical and compositional modulations to achieve the control of the magnetization reversal along with the nano-entities and, thus, enable the fabrication of spintronic, magnetic data storage, and sensing devices, among others. In this work, diameter-modulated FeNi nanowires are fabricated paying special effort to obtain sharp transition regions between two segments of different diameters (from about 450 nm to 120 nm), enabling precise control over the magnetic behavior of the sample. Micromagnetic simulations performed on single bi-segmented nanowires predict a double step magnetization reversal where the wide segment magnetization switches near 16 kA/m through a vortex domain wall, while at 40 kA/m the magnetization of the narrow segment is reversed through a corkscrew-like mechanism. Finally, these results are confirmed with magneto-optic Kerr effect measurements at the transition of isolated bi-segmented nanowires. Furthermore, macroscopic vibrating sample magnetometry is used to demonstrate that the magnetic decoupling of nanowire segments is the main phenomenon occurring over the entire fabricated nanowires.