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Glasslike Dynamics of Polar Domain Walls in Cryogenic SrTiO_{3}
David Pesquera1, Michael A Carpenter1, Ekhard K H Salje1
1Department of Earth Sciences, University of Cambridge, Downing Street, Cambridge CB2 3EQ, United Kingdom.
Abstract:
Polar and highly mobile domain walls in SrTiO_{3} move under electric and elastic fields. Two vastly different timescales dominate their dynamical behavior. The previously observed fast changes lead to anomalies near 40 K where the elastic moduli soften and the polarity of the walls becomes strong. Keeping the sample under isothermal conditions leads to a new and unexpected phenomenon: The softening vanishes over timescales of days while the piezoelectricity of the sample remains unchanged. The hardening follows glass dynamics below an onset at T^{*}≈40 K. The timescale of the hardening is strongly temperature dependent and can be followed experimentally down to 34 K when the relaxation is not completed within two days. The relaxation time of a stretched exponential decay increases exponentially with the decreasing temperature. This relaxation process follows similar dynamics after zero-field cooling and after applying or removing an electric field. The sluggish behavior is attributed to collective interactions of domain patterns following overdamped glass dynamics rather than ballistic dynamics.
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