Dual-comb spectroscopy of methane based on a free-running Erbium-doped fiber laser

Dual-comb spectroscopy has been developed into a high-precision technique that is capable of sensing many important species of samples, such as methane. Recent studies on single-cavity, dual-comb light sources further reduce the system complexity of such schemes. In contrast to the previous demonstrations around the lasing spectrum, this work significantly expands the spectral coverage of a dual-comb spectroscopy setup using one free-running laser to a region far beyond the laser's emission wavelengths. Nonlinear wavelength conversion based on soliton self-frequency shift is adopted to convert and tune the wavelengths of both dual-comb pulses to ~1650nm. It is shown that this process has introduced little additional intensity noise. The 2ν₃ absorption band of methane from 1647 nm to 1663nm is measured with very good agreement with HITRAN, and the standard deviation of the residual is < ~0.006 after averaging ~1.96 seconds of data. Our results further elucidate the potential of dual-comb spectroscopy using one laser, and could pave the way for the development of low-cost, power-efficient, and compact dual-comb instrument targeting more spectral regions.