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Extraction and Characterization of Surfactants from Atmospheric Aerosols
Published on: April 21, 2017
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Weak average liquid-cloud-water response to anthropogenic aerosols
Velle Toll1,2, Matthew Christensen3, Johannes Quaas4
1Department of Meteorology, University of Reading, Reading, UK. velle.toll@ut.ee.
Nature
|August 2, 2019
Summary
Anthropogenic aerosols cause a weak decrease in cloud water, contrary to previous theories. This finding reduces uncertainty in climate change projections by showing aerosols have a smaller cooling effect than expected.
Area of Science:
- Atmospheric Science
- Climate Science
- Cloud Physics
Background:
- Anthropogenic aerosols influence Earth's climate by interacting with clouds.
- Aerosol-induced cloud water increases, via suppressed rain, were hypothesized to cause significant cooling.
- This implied high sensitivity of surface temperature to anthropogenic forcing.
Purpose of the Study:
- To provide direct observational evidence of aerosol effects on cloud water.
- To quantify the impact of aerosols on liquid-phase cloud water content.
- To reassess the climate cooling effect attributed to aerosols.
Main Methods:
- Direct observation of polluted clouds downwind of various anthropogenic sources.
- Comparison of cloud water content in polluted versus unpolluted clouds.
- Estimation of aerosol-induced changes in cloud water and their contribution to climate forcing.
Main Results:
- Aerosols cause a relatively weak average decrease in liquid-phase cloud water.
- Aerosol effects of suppressed rain (increasing water) and enhanced evaporation (decreasing water) partially cancel.
- Observed cloud water decrease offsets 23% of the cooling effect from increased cloud droplet concentration.
Conclusions:
- The hypothesis of substantial climate cooling due to increased cloud water is invalidated.
- Aerosol-cloud interactions have a weaker cooling effect than previously estimated.
- Uncertainty in future climate projections is reduced.
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