Ramsey-Bordé Matter-Wave Interferometry for Laser Frequency Stabilization at 10^{-16} Frequency Instability and Below

We demonstrate Ramsey-Bordé (RB) atom interferometry for high performance laser stabilization with fractional frequency instability <2×10^{-16} for timescales between 10 and 1000s. The RB spectroscopy laser interrogates two counterpropagating ^{40}Ca beams on the ^{1}S_{0}-^{3}P_{1} transition at 657 nm, yielding 1.6 kHz linewidth interference fringes. Fluorescence detection of the excited state population is performed on the (4s4p) ^{3}P_{1}-(4p^{2}) ^{3}P_{0} transition at 431 nm. Minimal thermal shielding and no vibration isolation are used. These stability results surpass performance from other thermal atomic or molecular systems by 1 to 2 orders of magnitude, and further improvements look feasible.