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Related Concept Videos

Interfacial Electrochemical Methods: Overview01:06

Interfacial Electrochemical Methods: Overview

760
Interfacial electrochemical methods focus on the phenomena occurring at the boundary between an electrode and a solution, as opposed to bulk methods that concentrate on the solution's overall properties. These interfacial methods are classified as either static or dynamic based on the presence of a nonzero current in the electrochemical cell and the consistency of analyte concentrations. Static methods, such as potentiometry, measure the cell's potential without any significant current...
760

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Anisotropically Electrochemical-Mechanical Evolution in Solid-State Batteries and Interfacial Tailored Strategy.

Nan Sun1, Qingsong Liu1, Yi Cao1

  • 1MIIT Key Laboratory of Critical Materials Technology for New Energy Conversion and Storage, School of Chemistry and Chemical Engineering, Harbin Institute of Technology, Harbin, 150001, China.

Angewandte Chemie (International Ed. in English)
|October 15, 2019
PubMed
Summary

Solid-state batteries face challenges due to interface issues. This study reveals how interfacial changes and contact loss hinder performance, proposing in-situ electrolyte growth for robust solid-solid interfaces in advanced batteries.

Keywords:
electrochemistryinterfaceslithiumsolid-state batteriessulfide electrolyte

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Area of Science:

  • Materials Science
  • Electrochemistry
  • Energy Storage

Background:

  • All-solid-state batteries offer high energy density and safety advantages.
  • Practical application of solid-state batteries is limited by solid-solid interface issues.
  • Understanding electrode-electrolyte interface behavior is critical but challenging.

Purpose of the Study:

  • To fundamentally elucidate electrode-electrolyte interface behaviors in solid-state batteries.
  • To identify the mechanisms behind interfacial resistance and capacity fading.
  • To propose strategies for fabricating robust solid-solid interfaces.

Main Methods:

  • Probing interfacial resistance and capacity fading in solid-state batteries.
  • Analyzing heterogeneous phase transition evolution at solid-solid interfaces.
  • Investigating strain-induced interfacial changes and contact loss.

Main Results:

  • Heterogeneous phase transition evolution at solid-solid interfaces was revealed.
  • Strain-induced interfacial changes, contact loss, and dense metallic surface phases were identified as detrimental.
  • In-situ electrolyte growth on secondary particles was proposed as a method to create robust interfaces.

Conclusions:

  • The study provides fundamental insights into solid-solid interfacial reactions in solid-state batteries.
  • Understanding these mechanisms is crucial for optimizing advanced solid-state battery performance.
  • In-situ electrolyte growth offers a promising approach for enhancing interface stability.